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Structure Determination from Powder Diffraction Data$
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W.I.F. David, K. Shankland, L.B. McCusker, and C. Bärlocher

Print publication date: 2006

Print ISBN-13: 9780199205530

Published to Oxford Scholarship Online: January 2010

DOI: 10.1093/acprof:oso/9780199205530.001.0001

Extracting integrated intensities from powder diffraction patterns

Chapter:
(p. 136 ) 8 Extracting integrated intensities from powder diffraction patterns
Source:
Structure Determination from Powder Diffraction Data
Author(s):

William I.F. David

Devinderjit S.Sivia

Publisher:
Oxford University Press
DOI:10.1093/acprof:oso/9780199205530.003.0008

This chapter deals with the theoretical aspects of extracting integrated intensities from a powder diffraction pattern and with the ancillary issue of space group determination. Two principal methods are discussed: the iterative Le Bail method and the constrained linear least-squares approach of Pawley. The origins and mathematical basis of both methods are discussed and examples given to illustrate their performance on particular problems. The problems that occur in dealing with reflections that are strongly overlapping are considered and some methods for overcoming them suggested. A probabilistic basis for space group selection, based upon intensities extracted from a Pawley fit, is also given and illustrated with examples.

Keywords:   Le Bail method, Pawley fit, space group determination, space group extraction

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