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Nonlinear Optics and Photonics$
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Guang S. He

Print publication date: 2014

Print ISBN-13: 9780198702764

Published to Oxford Scholarship Online: December 2014

DOI: 10.1093/acprof:oso/9780198702764.001.0001

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Multi-Photon Nonlinear Optical Effects

Multi-Photon Nonlinear Optical Effects

(p.432) 14 Multi-Photon Nonlinear Optical Effects
Nonlinear Optics and Photonics

Guang S. He

Oxford University Press

According to the quantum theory of radiation, simultaneous multi-photon absorption by a single molecule could take place through a transition process involving intermediate state(s) of the combined system consisting of the input photon field and the molecule. The probability of the m (≥2)-photon absorption process is proportional to the mth power of the local light intensity. Based on this property, the highly multi-photon active materials and devices can be utilized to implement optical power limiting, optical stabilization and reshaping, and three-dimensional (3D) data storage and microfabrication. Moreover, based on the m-photon absorption induced frequency upconversion emission, researchers have realized high efficient m-photon pumped frequency upconversion lasing as well as frequency upconversion 3D scanning laser microscopy.

Keywords:   Multi-photon absorption, optical limiting, optical stabilization, optical reshaping, multi-photon pumped lasing, three-dimensional data storage, microfabrication, scanning laser microscopy

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